Dielectric barrier discharges (DBDs) offer great potential for applications such as volatile organic compounds (VOCs) conversion or plasma catalysis. For many of these applications, an admixture of molecular oxygen is important, for example, to oxidize the gases to be treated. However, oxygen addition can lead to a drastic change in discharge dynamics, which may affect conversion efficiency. The discharge may transition to a filamentary mode, which could influence plasma chemical processes or in extreme cases potentially damage the reactor. This study investigates the discharge mode of a micro cavity plasma array operated at atmospheric pressure with a helium flow (1-2slm) containing small oxygen admixtures (0-5%). A multitude of parameters as voltage, current, power, and emission are investigated for characterization. Additionally, the electric field, mean electron energy and atomic oxygen density are examined depending on the oxygen admixture. With pure helium, a homogeneous atmospheric pressure glow discharge (APGD) is observed, appearing as a quasi-continuous glow discharge. With small oxygen admixtures (0.1-1%), individual discharge pulses become visible, though they remain separated (pseudo glow discharge). At higher oxygen admixtures (>1%), a mode transition to a filamentary discharge is observed. The measurements indicate that the discharge mode, especially the individual discharge pulses, has a significant impact on conversion efficiency. This knowledge can help in the future to fine-tune the discharge mode using external parameters such as voltage waveform or frequency to optimize conversion efficiency.
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Release Date | 2024-11-28 |
Identifier | 8246146e-9880-4951-8c7b-4f12e8c3a675 |
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Plasma Source Properties | Voltage amplitudes of up to 800 V with a bipolar ramp frequency of 15 kHz are used. |
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Plasma Medium Properties | The reactor is operated at atmospheric pressure with a helium flow of 2 slm. In addition, molecular oxygen (0-50 sccm) as reactive admixture and argon (1 sccm) as actinometer gas can be added. |
Contact Name | David Steuer |
Contact Email | |
Public Access Level | Public |
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Data and Resources
- Figure2csv
Voltage, current and emission characteristics for ramp excitation under pure...
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Mean cavity filling depending on the oxygen admixture. Conditions: V = 1200V...
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Integrated emission of a single cavity depending on the oxygen admixture....
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Number of peaks (a), the intensity ratio of maximum to mean value (b) and...
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Power depending on the applied voltage for different oxygen admixtures (a)...
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Power depending on the applied voltage for different oxygen admixtures (a)...
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Fit of the 492nm helium line pair within the DPP to determine the electric...
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Fit of the 492nm helium line pair within the DPP to determine the electric...
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Electric field and fraction of the field-free line depending on the oxygen...
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Atomic oxygen density and mean electron energy as a function of O2-admixture...
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Atomic oxygen density for a single cavity as a function of time. Conditions...
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